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This book presents an in-depth overview of various electrolytes for electrochemical supercapacitors. The effects of the electrolyte properties on the performance of electrochemical supercapacitors are analyzed in depth. The principles and methods to design and optimize the electrolytes for electrochemical supercapacitors are highlighted through extensive analysis of the literature. The interplay between the electrolytes and active electrode materials and inactive components (current collectors, binders, and separators) are discussed. This is concluded by the challenges they presently face and the outlook for their future use.